Watchmen and V for Vendetta? No, I'm not horribly biased. Hell, might as well throw Mushishi in there too, since it doesn't have an overarching plot and any episode can stand on its own.
Sherlock Holmes (/still hasn't seen it)
Baccano! was discussed earlier...

Maybe some lame/silly/badly dubbed movies too for fun. old crappy animes or cheesy kung fu. lol...